Spin Glass Transition at Nonzero Temperature in a Disordered Dipolar Ising System: The Case of LiHoxY{1-x}F4

TL;DR

This paper provides strong computational evidence that a spin glass transition occurs at nonzero temperature in a realistic model of LiHo$_{x}$Y$_{1-x}$F$_{4}$, a disordered dipolar Ising system, resolving a long-standing debate.

Contribution

The study demonstrates, through extensive simulations, the existence of a spin glass transition at finite temperature in a realistic microscopic model of LiHo$_{x}$Y$_{1-x}$F$_{4}$, a key experimental system.

Findings

Evidence of nonzero temperature spin glass transition in simulations.

Confirmation that dipolar interactions lead to spin glass behavior.

Resolution of controversy regarding spin glass transition in disordered dipolar systems.

Abstract

The physics of the spin glass (SG) state, with magnetic moments (spins) frozen in random orientations, is one of the most intriguing problems in condensed matter physics. While most theoretical studies have focused on the Edwards-Anderson model of Ising spins with only discrete `up/down' directions, such Ising systems are experimentally rare. LiHo$_{x}$Y$_{1-x}$F$_{4}$, where the Ho$^{3+}$ moments are well described by Ising spins, is an almost ideal Ising SG material. In LiHo$_{x}$Y$_{1-x}$F$_{4}$, the Ho$^{3+}$ moments interact predominantly via the inherently frustrated magnetostatic dipole-dipole interactions. The random frustration causing the SG behavior originates from the random substitution of dipole-coupled Ho$^{3+}$ by non-magnetic Y$^{3+}$. In this paper, we provide compelling evidence from extensive computer simulations that a SG transition at nonzero temperature occurs in a realistic microscopic model of LiHo$_{x}$Y$_{1-x}$F$_{4}$, hence resolving the long-standing, and still ongoing, controversy about the existence of a SG transition in disordered dipolar Ising systems.