X-ray refractive index of laser-dressed atoms

TL;DR

This paper develops an ab initio quantum electrodynamics theory to calculate the x-ray refractive index of laser-dressed atoms, demonstrating phenomena like electromagnetically induced transparency in argon near the K edge.

Contribution

It introduces a nonperturbative method to compute the x-ray refractive index of laser-dressed atoms, enabling new control over x-ray pulse shaping and transparency.

Findings

Demonstrated electromagnetically induced transparency (EIT) for x rays in argon.

Showed laser dressing modifies the x-ray polarizability and absorption.

Enabled imprinting ultrafast laser pulse shapes onto x-ray pulses.

Abstract

We investigated the complex index of refraction in the x-ray regime of atoms in laser light. The laser (intensity up to 10^13 W/cm^2, wavelength 800nm) modifies the atomic states but, by assumption, does not excite or ionize the atoms in their electronic ground state. Using quantum electrodynamics, we devise an ab initio theory to calculate the dynamic dipole polarizability and the photoabsorption cross section, which are subsequently used to determine the real and imaginary part, respectively, of the refractive index. The interaction with the laser is treated nonperturbatively; the x-ray interaction is described in terms of a one-photon process. We numerically solve the resolvents involved using a single-vector Lanczos algorithm. Finally, we formulate rate equations to copropagate a laser and an x-ray pulse through a gas cell. Our theory is applied to argon. We study the x-ray polarizability and absorption near the argon K edge over a large range of dressing-laser intensities. We find electromagnetically induced transparency (EIT) for x rays on the Ar 1s --> 4p pre-edge resonance. We demonstrate that EIT in Ar allows one to imprint the shape of an ultrafast laser pulse on a broader x-ray pulse (duration 100ps, photon energy 3.2keV). Our work thus opens new opportunities for research with hard x-ray sources.