Coinage-metal capping effects on the spin-reorientations of Co/Ru(0001)

TL;DR

This study investigates how coinage-metal capping layers influence the spin reorientation transition and magnetic anisotropy in Co/Ru(0001) thin films, revealing material-dependent effects and conditions for high perpendicular magnetic anisotropy.

Contribution

It provides real-space observations of SRT modifications due to coinage-metal capping and explains these effects through ab-initio calculations, highlighting new ways to enhance magnetic anisotropy.

Findings

Capping modifies the SRT depending on material and thickness.

Quantitative enhancement of magnetic anisotropy observed.

Conditions for high perpendicular magnetic anisotropy identified.

Abstract

Thin films of Co/Ru(0001) are known to exhibit an unusual spin reorientation transition (SRT) coupled to the completion of Co atomic layers for Co thicknesses under 4 layers. By means of spin-polarized low-energy electron microscopy, we follow in real space the magnetization orientation during the growth of atomically thick capping layers on Co/Ru(0001). Capping with coinage-metal (Cu, Ag, Au) elements modifies the SRT depending on the Co and overlayer thickness and on the overlayer material, resulting in an expanded range of structures with high perpendicular magnetic anisotropy. The origin of the SRT can be explained in terms of ab-initio calculations of the layer-resolved contributions to the magnetic anisotropy energy. Besides the changes in the SRT introduced by the capping, a quantitative enhancement of the magnetic anisotropy is identified. A detailed analysis of the interplay between strain and purely electronic effects allows us to identify the conditions that lead to a high perpendicular magnetic anisotropy in thin hcp Co films.