Small angle neutron scattering study of the step-like magnetic transformation in Pr0.70Ca0.30MnO3

TL;DR

This study uses small angle neutron scattering to investigate the magnetic phase transformations in Pr0.7Ca0.3MnO3, revealing a temperature-dependent transition from continuous to step-like phase changes involving ferromagnetic and insulating phases.

Contribution

It provides new insights into the mesoscopic magnetic domain formation and the role of elastic strain relaxation in phase transformations at low temperatures.

Findings

Step-like magnetic transformation observed below 5K.

Formation of ferromagnetic metallic domains within insulating phases.

Elastic strain relaxation influences phase transition mechanisms.

Abstract

Small angle neutron scattering (SANS) magnetic and electrical transport measurements were performed to study a single crystal of Pr0.7Ca0.3MnO3, a colossal magnetoresistive (CMR) material. While the magnetic field induced transformation of this phase separated compound consisting of an antiferromagnetic insulating phase (AFI) and a ferromagnetic insulating phase (FI), is continuous at high temperature (above 5K), at lower temperature a step like transformation is observed (around 5T at 2K). Macroscopic magnetization measurements and SANS indicate that this transformation occurs by the formation of mesoscopic ferromagnetic metallic (FM) domains in the AFI phase, and, eventually, in the FI phase. Although above 5K this transformation is continuous, below 5K a magnetization step marks the abrupt transition from a large scale FI/AFI phase separation to a large scale phase separation between AFI, FI and FM phases. Our results suggest that relaxation of elastic strains inherent to the coexistence of these different phases plays a crucial role in the mechanism of these transformations. The occurrence of magnetization steps could result from an intrinsic behavior of the AFI phase at low temperature.