Crossover from Kondo assisted suppression to co-tunneling enhancement of tunneling magnetoresistance via ferromagnetic nanodots in MgO tunnel barriers

TL;DR

This study investigates how magnetic nanodots within MgO tunnel barriers influence tunneling magnetoresistance, revealing a crossover from Kondo-assisted suppression to co-tunneling enhancement at different nanodot sizes and temperatures.

Contribution

It demonstrates the transition in TMR behavior caused by nanodot size and Coulomb blockade effects in MgO-based magnetic tunnel junctions.

Findings

Kondo-assisted tunneling increases conductance at low bias for thin nanodots.

TMR is suppressed in the Coulomb blockade regime for small nanodots.

TMR is enhanced via co-tunneling for larger nanodots.

Abstract

Recently, it has been shown that magnetic tunnel junctions with thin MgO tunnel barriers exhibit extraordinarily high tunneling magnetoresistance (TMR) values at room temperature1, 2. However, the physics of spin dependent tunneling through MgO barriers is only beginning to be unravelled. Using planar magnetic tunnel junctions in which ultra-thin layers of magnetic metals are deposited in the middle of a MgO tunnel barrier here we demonstrate that the TMR is strongly modified when these layers are discontinuous and composed of small pancake shaped nanodots. At low temperatures, in the Coulomb blockade regime, for layers less than ~1 nm thick, the conductance of the junction is increased at low bias consistent with Kondo assisted tunneling. In the same regime we observe a suppression of the TMR. For slightly thicker layers, and correspondingly larger nanodots, the TMR is enhanced at low bias, consistent with co-tunneling.