Thermal and surface anisotropy effects on the magnetization reversal of a nanocluster

TL;DR

This paper investigates how surface anisotropy influences the magnetization reversal process in magnetic nanoclusters, revealing significant effects on relaxation rates and switching fields, and proposes experimental comparisons for surface anisotropy insights.

Contribution

It introduces an effective anisotropy model to analyze surface anisotropy effects on magnetization reversal in nanoclusters, highlighting deviations from classical models.

Findings

Surface anisotropy can alter reversal rates by over an order of magnitude.

Temperature-dependent switching fields deviate from the Stoner-Wohlfarth model.

Comparison with $$-SQUID data can reveal surface anisotropy properties.

Abstract

The relaxation rate and temperature-dependent switching field curve of a spherical magnetic nanocluster are calculated by taking into account the effect of surface anisotropy via an effective anisotropy model. In particular, it is shown that surface anisotropy may change the thermally activated magnetization reversal by more than an order of magnitude, and that temperature-dependent switching field curves noticeably deviate from the Stoner-Wohlfarth astroid. With recent and future $\mu$-SQUID measurements in mind, we indicate how comparison of our results with experimental data on isolated clusters may allow one to obtain valuable information on surface anisotropy.