Methods for analytically estimating the resolution and intensity of neutron time-of-flight spectrometers. The case of the TOFTOF spectrometer

TL;DR

This paper presents an analytical approach to estimate the energy resolution and intensity of the TOFTOF neutron spectrometer, aiding users in optimizing instrument parameters for quasi-elastic neutron scattering studies.

Contribution

It adapts a previously successful analytical method to the high-resolution TOFTOF spectrometer, providing detailed calculations and graphical tools for parameter optimization.

Findings

Resolution and intensity depend on neutron wavelength, chopper speed, and frame overlap ratio.

Graphs of iso-resolution and iso-intensity lines assist in instrument configuration.

Alternative frame overlap ratio options are discussed for different dynamical ranges.

Abstract

An analytical method is presented with allows to estimate the energy resolution of time-of-flight neutron spectrometers, as well as its partial contributions, over a dynamical range that extends from the elastic line to the accessible inelastic regions. Such a method, already successfully applied in the past to the TOSCA and HET neutron inelastic scattering spectrometers installed at the ISIS neutron spallation source [A M Gaspar, PhD Thesis, Universidade Tecnica de Lisboa, 2004], is here applied to the high resolution time-of-flight spectrometer TOFTOF, mainly dedicated to quasi-elastic neutron scattering studies and installed at the new neutron reactor FRM II. To make such calculations easily understandable, the principle of work of the TOFTOF instrument and of each of its components is explained in detail. A simply method that can be used to estimate the instrument intensity, i.e. of the number of neutrons arriving at the sample position per unit time, is also briefly outlined. To the benefit of the TOFTOF users, graphs displaying the dependencies of the instrument resolution at the elastic line and of the instrument intensity on the relevant instrument parameters, i.e the wavelength of the incident neutrons, the choppers speed of rotation and the frame overlap ratio, are presented, in the form of iso-resolution or iso-intensity lines. The method of estimation of the frame overlap ratio that is commonly used at time-of-flight instruments such as TOFTOF is also explained and alternative options concerning this parameter, depending on the dynamical range of interest, are briefly addressed.