Shear thickening of cornstarch suspensions as a re-entrant jamming transition

TL;DR

This paper investigates the shear thickening behavior of cornstarch suspensions, revealing a re-entrant jamming transition driven by confinement and dilation effects, with implications for understanding dense suspension rheology.

Contribution

It demonstrates that shear thickening in cornstarch suspensions results from a re-entrant jamming transition linked to Reynolds dilatancy and confinement effects.

Findings

Shear thickening correlates with a jamming transition.

The onset shear rate depends on the shear cell gap.

Dilation under shear is confirmed as a key factor.

Abstract

We study the rheology of cornstarch suspensions, a dense system of non-Brownian particles that exhibits shear thickening, i.e. a viscosity that increases with increasing shear rate. Using MRI velocimetry we show that the suspension has a yield stress. From classical rheology it follows that as a function of the applied stress the suspension is first solid (yield stress), then liquid and then solid again when it shear thickens. The onset shear rate for thickening is found to depend on the measurement geometry: the smaller the gap of the shear cell, the lower the shear rate at which thickening occurs. Shear thickening can then be interpreted as the consequence of the Reynolds dilatancy: the system under flow wants to dilate but instead undergoes a jamming transition because it is confined, as confirmed by measurement of the dilation of the suspension as a function of the shear rate.