Observation of strong-coupling effects in a diluted magnetic semiconductor (Ga,Fe)N

TL;DR

This paper reports the direct observation of strong-coupling effects in a (Ga,Fe)N diluted magnetic semiconductor, revealing giant Zeeman splitting and insights into p-d hybridization effects on exchange interactions.

Contribution

It provides the first direct measurement of giant Zeeman splitting in (Ga,Fe)N and demonstrates the impact of strong p-d hybridization on exchange energy renormalization.

Findings

Giant Zeeman splitting observed in (Ga,Fe)N

Ferromagnetic sign of exchange interactions confirmed

Reduced magnitude of effective p-d exchange energy

Abstract

A direct observation of the giant Zeeman splitting of the free excitons in (Ga,Fe)N is reported. The magnetooptical and magnetization data imply the ferromagnetic sign and a reduced magnitude of the effective p-d exchange energy governing the interaction between Fe^{3+} ions and holes in GaN, N_0 beta^(app) = +0.5 +/- 0.2 eV. This finding corroborates the recent suggestion that the strong p-d hybridization specific to nitrides and oxides leads to significant renormalization of the valence band exchange splitting.