Spin relaxation in $n$-type GaAs quantum wells with transient spin grating

TL;DR

This paper uses kinetic spin Bloch equations to analyze transient spin grating in GaAs quantum wells, revealing detailed spin relaxation and transport properties, and providing improved methods to extract key parameters from experimental data.

Contribution

It introduces a comprehensive theoretical framework for analyzing spin relaxation and transport in GaAs quantum wells using transient spin grating, including Coulomb effects and accurate parameter extraction methods.

Findings

Spin signal decays double exponentially with two rates.

Quadratic relation between decay rates and wave-vector at high temperature.

Coulomb drag significantly affects spin diffusion coefficient.

Abstract

By solving the kinetic spin Bloch equations, we study the time evolution of the transient spin grating, whose spin polarization varies periodically in real space, confined in (001) GaAs quantum wells. With this study we can investigate the properties of both the spin transport and the spin relaxation at the same time. The Fourier component of the spin signal decays double exponentially with two decay rates $1/\tau_+$ and $1/\tau_-$. In high temperature regime, the average of these two rates varies with the grating wave-vector $q$ quadratically, i.e., $(1/\tau_++1/\tau_-)/2=D_sq^2+1/\tilde{\tau}_s$, with $D_s$ and $\tilde{\tau}_s$ representing the spin diffusion coefficient and the average of the out-of-plane and the in-plane spin relaxation times respectively. $\tau_{\pm}$ calculated from our theory are in good agreement with the experimental data by Weber {\em et al.} [Phys. Rev. Lett. {\bf 98}, 076604 (2007)]. By comparing $D_s$ with and without the electron-electron Coulomb scattering, we calculate the contribution of Coulomb drag to the spin diffusion coefficient. With the transient spin grating result, we further reveal the relations among different characteristic parameters such as spin diffusion coefficient $D_s$, spin relaxation time $\tau_s$, and spin injection length $L_s$. We show that in the presence of the Dresselhaus and/or Rashba spin-orbit coupling, the widely used relation $L_s=\sqrt{D_s\tau_s}$ is generally inaccurate and can even be very wrong in some special cases. We present an accurate way to extract the steady-state transport characteristic parameters from the transient spin grating signals.