Coherent Electron Scattering Captured by an Attosecond Quantum Stroboscope

TL;DR

This paper introduces an attosecond quantum stroboscope that captures and images the full three-dimensional motion of electrons on a sub-femtosecond timescale, advancing ultrafast electron dynamics measurement.

Contribution

It presents a novel technique using synchronized attosecond pulse trains and a velocity map imaging spectrometer to guide and image electron scattering events in real time.

Findings

Successfully guided ionized electrons back to their parent ions.

Captured high-resolution images of electron scattering events.

Demonstrated control over electron motion on a sub-femtosecond scale.

Abstract

The basic properties of atoms, molecules and solids are governed by electron dynamics which take place on extremely short time scales. To measure and control these dynamics therefore requires ultrafast sources of radiation combined with efficient detection techniques. The generation of extreme ultraviolet (XUV) attosecond (1 as = 10-18 s) pulses has, for the first time, made direct measurements of electron dynamics possible. Nevertheless, while various applications of attosecond pulses have been demonstrated experimentally, no one has yet captured or controlled the full three dimensional motion of an electron on an attosecond time scale. Here we demonstrate an attosecond quantum stroboscope capable of guiding and imaging electron motion on a sub-femtosecond (1 fs = 10-15 s) time scale. It is based on a sequence of identical attosecond pulses which are synchronized with a guiding laser field. The pulse to pulse separation in the train is tailored to exactly match an optical cycle of the laser field and the electron momentum distributions are detected with a velocity map imaging spectrometer (VMIS). This technique has enabled us to guide ionized electrons back to their parent ion and image the scattering event. We envision that coherent electron scattering from atoms, molecules and surfaces captured by the attosecond quantum stroboscope will complement more traditional scattering techniques since it provides high temporal as well as spatial resolution.