Microscopic theory of quantum dot interactions with quantum light: local field effect

TL;DR

This paper develops a microscopic theory for the electromagnetic response of a quantum dot interacting with quantum light, incorporating local-field effects, and predicts novel phenomena in Rabi oscillations and absorption spectra.

Contribution

It introduces a new microscopic Hamiltonian model that accounts for depolarization and local-field effects in quantum dot-light interactions, extending the Jaynes-Cummings framework.

Findings

Prediction of two oscillatory regimes in Rabi effect with bifurcation.

Distortion of collapse-revival phenomena in quantum dot population inversion.

Appearance of a fine structure in the absorption spectrum due to local-field effects.

Abstract

A theory of both linear and nonlinear electromagnetic response of a single QD exposed to quantum light, accounting the depolarization induced local--field has been developed. Based on the microscopic Hamiltonian accounting for the electron--hole exchange interaction, an effective two--body Hamiltonian has been derived and expressed in terms of the incident electric field, with a separate term describing the QD depolarization. The quantum equations of motion have been formulated and solved with the Hamiltonian for various types of the QD excitation, such as Fock qubit, coherent fields, vacuum state of electromagnetic field and light with arbitrary photonic state distribution. For a QD exposed to coherent light, we predict the appearance of two oscillatory regimes in the Rabi effect separated by the bifurcation. In the first regime, the standard collapse--revivals phenomenon do not reveal itself and the QD population inversion is found to be negative, while in the second one, the collapse--revivals picture is found to be strongly distorted as compared with that predicted by the standard Jaynes-Cummings model. %The model developed can easily be extended to %%electromagnetic excitation. For the case of QD interaction with arbitrary quantum light state in the linear regime, it has been shown that the local field induce a fine structure of the absorbtion spectrum. Instead of a single line with frequency corresponding to which the exciton transition frequency, a duplet is appeared with one component shifted by the amount of the local field coupling parameter. It has been demonstrated the strong light--mater coupling regime arises in the weak-field limit. A physical interpretation of the predicted effects has been proposed.